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Rhonda Wellington Lloyd, a rich yuppie girl, self-proclaimed fashion queen
Brooke Lloyd, her mother
Buckley Lloyd, her father

Lila Sawyer, a nice girl who came from a farming community, Arnold's crush. However, she only prefers Arnold as a friend.
Lila's Father
 
Stinky Peterson, lanky boy from Arkansas, has a southern accent and a love for lemon pudding.
Stinky's father
Stinky's grandparents
Uncle Stinky

Eugene Horowitz, a geeky, nerdy, optimistic boy, the class jinx. He is often bullied.
Nate Horowitz, his father
Mrs. Horowitz, his mother
 
Sid, a boy with paranoid tendencies
Ray, his father
Sid's mother (Only appears in Parents' Day" and "On the Lam" )

Thaddeus "Curly" Gammelthorpe, the class' psychopath.
Curly's father
 

Torvald, the oldest boy in class who was tutored by Arnold
Torvald's mother

Sheena, nerdy girl who does not like violence
Sheena's uncle Earl, a boatman
Sheena's aunt Shelley, the school nurse

Lorenzo, a wealthy Hispanic American boy who does not have enough time to be a kid
Lorenzo's mother

Iggy, a kid that was popular until his classmates found out he wears bunny pajamas in "Arnold Betrays Iggy".
Iggy's mother
 
Brainy, a geek, Helga's stalker, usually knocked unconscious by Helga without Helga looking at him. Breathes noisily.
Nadine, young entomologist, Rhonda's best friend
Park, a close friend of Arnold and others. In the episode "Longest Monday" it is revealed he has a secret hide out.
Robert
Peapod Kid (He got his name from the "Downtown as Fruits" episode. He was a pea pod in the play.) He appears to be rich and possesses an eloquent vocabulary.
Joey Stevenson
Grandpa Phil also was Arnold's classmate in "Back to School" episode.
 
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Other students of PS 118 and their families
Billy
Big Gino, the boss of the school mafia
Camp Fire Lass, a girl who sells chocolate turtles, speaks with a Scottish accent
Chocolate Boy, a boy obsessed with chocolate. In "Chocolate Boy", it's revealed he eats chocolate because his nanny who he loved so much left him a bag of chocolate when she had to move a "far foreign land called Delaware". Arnold helps break Chocolate Boy of his obsession, but he only becomes as equally over-excessive eating radishes as a replacement.
Connie, a sixth grade girl who "dated" Gerald; Maria's best friend
Edmund, Wolfgang's sidekick
Gloria, a girl who looks like Helga, but has nicer personality
Maria, a sixth grade girl who "dated" Arnold; Connie's best friend
Maria's father
 
Mary, one of Big Patty's victims
Mickey the Weasel, a fifth grader
Wolfgang, the main bully of the block, a fifth grader
Katrinka
Ludwig, a bully, Wolfgang's rival
Ruth P. McDougal, a sixth grade girl, Arnold's first crush
Siobhan, an incredibly smart third grade girl
Simone, a sixth grade girl
Big Patty (Patty Smith), an ill-tempered sixth grade girl, Harold's friend.
Patty's mother Mother of Patty; short
Patty's father Father of Patty; also short.
 
Workers of PS 118 and their families
Dr. Bliss, a child psychologist who worked in the school for a day and later became Helga's psychoanalyst
Miss Felter, a substitute teacher, Arnold's crush
Mr. Frank, a sixth grade teacher
Lieutenant Major Goose, Arnold's teacher for short time (after Miss Slovak and before Mr. Simmons), a martinet. He also was Johanssen's drill sergeant during Vietnam War in "Veterans Day" episode
Lunch lady
Mr. Packenham, a fifth grade teacher
Sheena's aunt Shelley, the school nurse (already mentioned above)
Miss Slovak, Arnold's enthusiastic teacher (in the first season). She left teaching to pursue a career at golf.
Mr. Robert Simmons, Arnold's sensitive and caring teacher (since second season). Replaced Miss Slovak.
Principal Wartz, the strict, yet open-hearted principal of the school.
Coach Jack Wittenberg (voiced by Jim Belushi), the competitive school coach of many sports teams, which he often gets Arnold and his friends to join.
Tish Wittenberg, his wife, the coach of girls teams
Tucker Wittenberg, his son, a student of PS 118
Olga Pataki was Mr. Simmons's assistant in "Student Teacher" episode.
 
Other characters and their families
Mr. Bailey, a worker of the Hall of Records. His first appearance was in the Christmas Special, where Arnold came to him to help find Mr. Huynh's daughter, Mai. His 2nd appearance was in the series' feature film, where he helps trying find the document of the "Tomato Incident". When he couldn't find it, he tells Arnold about a man who keeps all kinds of historic records. (voiced by Vincent Schiavelli)
Betty, Mr. Leichliter's old love
Madame Blanche, a gypsy who sells magic potions
Bridget, head of a secret organization (Hey Arnold!: The Movie)
Bunny, an ex-wife of Dino Spumoni's. When he "died," he said that he would leave "jack squat" in his will for her. (E.G. Dailey)
Caesar, a man who seems to have many jobs
Mr. Camacho, owner of El Patio, the restaurant where Mr. Hyunh works
Agatha Caulfield, Arnold's favorite author
Cecile, Arnold's penpal from France
Superintendent Chaplin (Jack Angel), an official who supervises schools in the city
Charice, a girl Jamie O was in love with
Chloe, the girl Gerald had a crush on, while she fell for his older brother
 
I think Stanley may be my favorite. He's so ignorant, and hates his job, and doesn't pay attention to anything xD Haha, I just love him. I remember when he did the most pushups or something to get out of work early xD GO STANLEY!
 
Mayor Dixie, a woman mayor of Hillwood. In Hey Arnold!: The Movie, she allowed Scheck to redevelop Arnold's neighborhood, even though the city council rejected the idea. When she is shown Scheck destroying the document of the "Tomato Incident", she decides to make it a historic landmark once again.
Ray Doppel, an impersonator of Dino Spumoni
Eduardo, a friend of Arnold's parents who asked them to come to San Lorenzo
Floyd, an owner of a bar in countryside
Frankie G. and his gang: Tony B., Phily D., Joey C., and Chas, are a group of gang members
Councilman Gladhand, a member of the city council, lost his position to Marty Green (voiced by John O'Hurley)
Rabbi Goldberg, the Bermans' rabbi (voiced by Elliot Gould)
Councilman Marty Green, a dedicated butcher and a politician
Grubby man (voiced by Mark Hamill)
Harvey, a mailman (voiced by Lou Rawls)
Jacques, waiter at Chez Pierre restaurant
Davy Jones, a singer (voiced by Davy Jones himself)
Jimmy Kafka, Grandpa Phil's old friend and rival
Mickey Kaline, a retired baseball star and Arnold's favorite player. Arnold caught his final home run ball. (voiced by Ron Perlman)
Inge, German nanny hired by Patakis for short time
 
La Sombra, a villain who threatened the tribe of the Green Eyed
Leichliter, a dramatic critic and director
Lola, Ernie Potts's girlfriend (voiced by Jennifer Tilly)
Lucky, a fireman
Ronnie Matthews, Phoebe's favorite pop star who lip-synchs.
Maurice, actor who plays The Abdicator in a TV show
Monkeyman, a poor man who fights crime on the streets
Nashville Ned or Nocturnal Ned, the Radio DJ
Daniel Newton, documentary film director
Madame Parvenu, owner of a finishing school
Mona, Murray's girlfriend (Hey Arnold!: The Movie)
Murray, a bus driver and a war veteran (Hey Arnold!: The Movie)
Patrice, Charice's friend
Pigeon Man, a gentle outcast who preferred to associate with pigeons rather than people.
Pop Daddy, a character on a television show watched by Gerald and Arnold.
Pinkerton, Big Bob's employee
Officer Pudney, a woman officer of police
Sammy Redmond, a rich man who befriends Arnold
Alan Redmond, his son
 
Red, Mr. Scheck's assistant (Hey Arnold!: The Movie)
Revis and Jackie Lee, TV show hosts.
Don Reynolds, former Dino Spumoni's partner who wrote lyrics for him
Mr. Scheck (Alphonse Perrier du von Scheck), a developer who tried to tear down the neighborhood so he could build a mall (Hey Arnold!: The Movie)
Sandy, Summer's boyfriend
Sewer king, insane hermit who lives in the sewer
Fuzzy Slippers, Gerald's off-screen, but referenced, informant
Stoop Kid, kid who lives on a stoop and never leaves it
Summer, a girl Arnold met at the beach, and developed a crush on
Arnold Skelter, Miss Felter's boyfriend
Slim, a skilled mechanical bull rider
Rex Smythe-Higgins, old rival of Grandpa Phil
Rex Smythe-Higgins III, his grandson, Arnold's rival
Dino Spumoni, a Frank Sinatra-type singer, who faked suicide to increase his fame, but became angry with his subsequent impersonators.
Candy Maldonado, Dino's most recent ex-wife (fifth one)
Jimmy Maldonado, Candy's son
 
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