Go to the Podcast section of iTunes. Expand each Podcast and remove the check mark from any Podcast episode you no longer want. If you don't want a Podcast series at all then just right click on the Podcast Title and go to Delete and this will remove all episodes. Next time you sync they will be removed.
For Podcasts you want to keep downloading, right click on the name of the Podcast and select Allow Auto Delete. Then click the Settings button at the bottom of the screen and choose how many episodes you want iTunes to "Keep". Make sure to turn on Allow Auto Delete for all your Podcasts.
Make sure you're in the Podcast section of iTunes (not the Music section of your library).
There is a grey triangle to the left of each Podcast name pointing towards the name. Click on this and it will point down and you will see each episode listed below it.
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